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```rss https://www.springer.com/journal/40820 RSSHub i@diygod.me (DIYgod) zh-cn Tue, 10 Oct 2023 12:53:17 GMT 5 Green Vertical-Cavity Surface-Emitting Lasers Based on InGaN Quantum Dots and Short Cavity

Tao Yang; Yan-Hui Chen; Bao-Ping Zhang
https://doi.org/10.1007/s40820-023-01189-0
Volume 15, issue 1, December 2023

Room temperature low threshold lasing of green GaN-based vertical cavity surface emitting laser (VCSEL) was demonstrated under continuous wave (CW) operation. By using self-formed InGaN quantum dots (QDs) as the active region, the VCSEL emitting at 524.0 nm has a threshold current density of 51.97 A cm−2, the lowest ever reported. The QD epitaxial wafer featured with a high IQE of 69.94% and the δ-function-like density of states plays an important role in achieving low threshold current. Besides, a short cavity of the device (~ 4.0 λ) is vital to enhance the spontaneous emission coupling factor to 0.094, increase the gain coefficient factor, and decrease the optical loss. To improve heat dissipation, AlN layer was used as the current confinement layer and electroplated copper plate was used to replace metal bonding. The results provide important guidance to achieving high performance GaN-based VCSELs.

]]> https://link.springer.com/article/10.1007/s40820-023-01189-0 https://link.springer.com/article/10.1007/s40820-023-01189-0 High-Performance Silicon-Rich Microparticle Anodes for Lithium-Ion Batteries Enabled by Internal Stress Mitigation

Yao Gao; Lei Fan; Biao Zhang
https://doi.org/10.1007/s40820-023-01190-7
Volume 15, issue 1, December 2023

Si is a promising anode material for Li ion batteries because of its high specific capacity, abundant reserve, and low cost. However, its rate performance and cycling stability are poor due to the severe particle pulverization during the lithiation/delithiation process. The high stress induced by the Li concentration gradient and anisotropic deformation is the main reason for the fracture of Si particles. Here we present a new stress mitigation strategy by uniformly distributing small amounts of Sn and Sb in Si micron-sized particles, which reduces the Li concentration gradient and realizes an isotropic lithiation/delithiation process. The Si8.5Sn0.5Sb microparticles (mean particle size: 8.22 μm) show over 6000-fold and tenfold improvements in electronic conductivity and Li diffusivity than Si particles, respectively. The discharge capacities of the Si8.5Sn0.5Sb microparticle anode after 100 cycles at 1.0 and 3.0 A g−1 are 1.62 and 1.19 Ah g−1, respectively, corresponding to a retention rate of 94.2% and 99.6%, respectively, relative to the capacity of the first cycle after activation. Multicomponent microparticle anodes containing Si, Sn, Sb, Ge and Ag prepared using the same method yields an ultra-low capacity decay rate of 0.02% per cycle for 1000 cycles at 1 A g−1, corroborating the proposed mechanism. The stress regulation mechanism enabled by the industry-compatible fabrication methods opens up enormous opportunities for low-cost and high-energy–density Li-ion batteries.

]]> https://link.springer.com/article/10.1007/s40820-023-01190-7 https://link.springer.com/article/10.1007/s40820-023-01190-7 Humanoid Intelligent Display Platform for Audiovisual Interaction and Sound Identification

Yang Wang; Wenli Gao; Shengjie Ling
https://doi.org/10.1007/s40820-023-01199-y
Volume 15, issue 1, December 2023

This study proposes a rational strategy for the design, fabrication and system integration of the humanoid intelligent display platform (HIDP) to meet the requirements of highly humanized mechanical properties and intelligence for human–machine interfaces. The platform's sandwich structure comprises a middle light-emitting layer and surface electrodes, which consists of silicon elastomer embedded with phosphor and silk fibroin ionoelastomer, respectively. Both materials are highly stretchable and resilient, endowing the HIDP with skin-like mechanical properties and applicability in various extreme environments and complex mechanical stimulations. Furthermore, by establishing the numerical correlation between the amplitude change of animal sounds and the brightness variation, the HIDP realizes audiovisual interaction and successful identification of animal species with the aid of Internet of Things (IoT) and machine learning techniques. The accuracy of species identification reaches about 100% for 200 rounds of random testing. Additionally, the HIDP can recognize animal species and their corresponding frequencies by analyzing sound characteristics, displaying real-time results with an accuracy of approximately 99% and 93%, respectively. In sum, this study offers a rational route to designing intelligent display devices for audiovisual interaction, which can expedite the application of smart display devices in human–machine interaction, soft robotics, wearable sound-vision system and medical devices for hearing-impaired patients.

]]> https://link.springer.com/article/10.1007/s40820-023-01199-y https://link.springer.com/article/10.1007/s40820-023-01199-y Initiating Binary Metal Oxides Microcubes Electrsomagnetic Wave Absorber Toward Ultrabroad Absorption Bandwidth Through Interfacial and Defects Modulation

Fushan Li; Nannan Wu; Chuanxin Hou
https://doi.org/10.1007/s40820-023-01197-0
Volume 15, issue 1, December 2023

3D cubic hollow core–shell NiCo2O4@C composites were synthesized. Oxygen vacancies were introduced into the prepared composites. Ultrabroad effective absorption bandwidth of 12.48 GHz was obtained. The absorption performance mechanism of NiCo2O4/C composites was investigated.

]]> https://link.springer.com/article/10.1007/s40820-023-01197-0 https://link.springer.com/article/10.1007/s40820-023-01197-0 Effectively Modulating Oxygen Vacancies in Flower-Like δ-MnO2 Nanostructures for Large Capacity and High-Rate Zinc-Ion Storage

Yiwei Wang; Yuxiao Zhang; Zhenjiang Li
https://doi.org/10.1007/s40820-023-01194-3
Volume 15, issue 1, December 2023

In recent years, manganese-based oxides as an advanced class of cathode materials for zinc-ion batteries (ZIBs) have attracted a great deal of attentions from numerous researchers. However, their slow reaction kinetics, limited active sites and poor electrical conductivity inevitably give rise to the severe performance degradation. To solve these problems, herein, we introduce abundant oxygen vacancies into the flower-like δ-MnO2 nanostructure and effectively modulate the vacancy defects to reach the optimal level (δ-MnO2−x−2.0). The smart design intrinsically tunes the electronic structure, guarantees ion chemisorption–desorption equilibrium and increases the electroactive sites, which not only effectively accelerates charge transfer rate during reaction processes, but also endows more redox reactions, as verified by first-principle calculations. These merits can help the fabricated δ-MnO2−x−2.0 cathode to present a large specific capacity of 551.8 mAh g−1 at 0.5 A g−1, high-rate capability of 262.2 mAh g−1 at 10 A g−1 and an excellent cycle lifespan (83% of capacity retention after 1500 cycles), which is far superior to those of the other metal compound cathodes. In addition, the charge/discharge mechanism of the δ-MnO2−x−2.0 cathode has also been elaborated through ex situ techniques. This work opens up a new pathway for constructing the next-generation high-performance ZIBs cathode materials.

]]> https://link.springer.com/article/10.1007/s40820-023-01194-3 https://link.springer.com/article/10.1007/s40820-023-01194-3 MXene Lubricated Tribovoltaic Nanogenerator with High Current Output and Long Lifetime

Wenyan Qiao; Linglin Zhou; Jie Wang
https://doi.org/10.1007/s40820-023-01198-z
Volume 15, issue 1, December 2023

Successfully solves the key issue of tribovoltaic nanogenerators (TVNGs) lifetime (90,000 cycles) and improves its output current density (754 mA m−2) simultaneously. Conductive polar liquid with MXene as additive is proposed as the dominant factor in enhancing the electrical output performance and durability of TVNG simultaneously. The mechanism of lubricated TVNG with enhanced output performance is explained from the perspective of solution polarity at the first time. Mxene solution exhibits universality in different types of semiconductor systems (Cu and P-type Si, and Cu and N-GaAs as material pairs).

]]> https://link.springer.com/article/10.1007/s40820-023-01198-z https://link.springer.com/article/10.1007/s40820-023-01198-z Graphene Quantum Dot-Mediated Atom-Layer Semiconductor Electrocatalyst for Hydrogen Evolution

Bingjie Hu; Kai Huang; Liang Wang
https://doi.org/10.1007/s40820-023-01182-7
Volume 15, issue 1, December 2023

The functional groups on graphene quantum dots (GQDs) for boosting the formation of MoS2 nanosheets via theoretical calculations were predicted. Near atom-layer-QD@SO3 with about 2 nm were synthesized using a functionalized GQD-induced in-situ bottom-up approach. Mechanistic insight on the role of functionalized GQDs was elaborated, namely, electron-withdrawing group functionalized GQDs facilitate the formation of nanosheet architectures of MoS2 compared to electron-donating group.

]]> https://link.springer.com/article/10.1007/s40820-023-01182-7 https://link.springer.com/article/10.1007/s40820-023-01182-7 Artificial Macrophage with Hierarchical Nanostructure for Biomimetic Reconstruction of Antitumor Immunity

Henan Zhao; Renyu Liu; You-Nian Liu
https://doi.org/10.1007/s40820-023-01193-4
Volume 15, issue 1, December 2023

Artificial cells are constructed from synthetic materials to imitate the biological functions of natural cells. By virtue of nanoengineering techniques, artificial cells with designed biomimetic functions provide alternatives to natural cells, showing vast potential for biomedical applications. Especially in cancer treatment, the deficiency of immunoactive macrophages results in tumor progression and immune resistance. To overcome the limitation, a BaSO4@ZIF-8/transferrin (TRF) nanomacrophage (NMΦ) is herein constructed as an alternative to immunoactive macrophages. Alike to natural immunoactive macrophages, NMΦ is stably retained in tumors through the specific affinity of TRF to tumor cells. Zn2+ as an “artificial cytokine” is then released from the ZIF-8 layer of NMΦ under tumor microenvironment. Similar as proinflammatory cytokines, Zn2+ can trigger cell anoikis to expose tumor antigens, which are selectively captured by the BaSO4 cavities. Therefore, the hierarchical nanostructure of NMΦs allows them to mediate immunogenic death of tumor cells and subsequent antigen capture for T cell activation to fabricate long-term antitumor immunity. As a proof-of-concept, the NMΦ mimics the biological functions of macrophage, including tumor residence, cytokine release, antigen capture and immune activation, which is hopeful to provide a paradigm for the design and biomedical applications of artificial cells.

]]> https://link.springer.com/article/10.1007/s40820-023-01193-4 https://link.springer.com/article/10.1007/s40820-023-01193-4 Kinetic Limits of Graphite Anode for Fast-Charging Lithium-Ion Batteries

Suting Weng; Gaojing Yang; Xuefeng Wang
https://doi.org/10.1007/s40820-023-01183-6
Volume 15, issue 1, December 2023

The microstructure of graphite upon rapid Li+ intercalation is a mixture of differently staging structures in the macroscopic and microscopic scales due to the incomplete and inhomogeneous intercalation reactions hindered by the sluggish reaction kinetics. The Li+ interface diffusion dominates the reaction kinetics at high rates in thin graphite electrode, while Li+ diffusion through the electrode cannot to be neglected for thick graphite electrode.

]]> https://link.springer.com/article/10.1007/s40820-023-01183-6 https://link.springer.com/article/10.1007/s40820-023-01183-6 Micro–Nano Water Film Enabled High-Performance Interfacial Solar Evaporation

Zhen Yu; Yuqing Su; Shaoan Cheng
https://doi.org/10.1007/s40820-023-01191-6
Volume 15, issue 1, December 2023

Micro–nano water film enhanced interfacial solar evaporator enables a high evaporation rate of 2.18 kg m−2 h−1 under 1 sun. An outdoor device with an enhanced condensation design demonstrates a high water production rate of 15.9–19.4 kg kW−1 h−1 m−2. A multi-objective predictive model is established to assess outdoor water production performance.

]]> https://link.springer.com/article/10.1007/s40820-023-01191-6 https://link.springer.com/article/10.1007/s40820-023-01191-6 Recent Advances in Multifunctional Reticular Framework Nanoparticles: A Paradigm Shift in Materials Science Road to a Structured Future

Maryam Chafiq; Abdelkarim Chaouiki; Young Gun Ko
https://doi.org/10.1007/s40820-023-01180-9
Volume 15, issue 1, December 2023

This review summarizes the quarter-century of reticular chemistry. Preparation strategies and characterization of reticular framework nanoparticles (RF-NPs) are systematically reviewed. Biomedicine, gas valorization, energy storage and other newer applications of RF-NPs are involved Future potential and challenges of RF-NPs are prospected.

]]> https://link.springer.com/article/10.1007/s40820-023-01180-9 https://link.springer.com/article/10.1007/s40820-023-01180-9 Adsorption Site Regulations of [W–O]-Doped CoP Boosting the Hydrazine Oxidation-Coupled Hydrogen Evolution at Elevated Current Density

Ge Meng; Ziwei Chang; Jianlin Shi
https://doi.org/10.1007/s40820-023-01185-4
Volume 15, issue 1, December 2023

Hydrazine oxidation reaction (HzOR) assisted hydrogen evolution reaction (HER) offers a feasible path for low power consumption to hydrogen production. Unfortunately however, the total electrooxidation of hydrazine in anode and the dissociation kinetics of water in cathode are critically depend on the interaction between the reaction intermediates and surface of catalysts, which are still challenging due to the totally different catalytic mechanisms. Herein, the [W–O] group with strong adsorption capacity is introduced into CoP nanoflakes to fabricate bifunctional catalyst, which possesses excellent catalytic performances towards both HER (185.60 mV at 1000 mA cm−2) and HzOR (78.99 mV at 10,00 mA cm−2) with the overall electrolyzer potential of 1.634 V lower than that of the water splitting system at 100 mA cm−2. The introduction of [W–O] groups, working as the adsorption sites for H2O dissociation and N2H4 dehydrogenation, leads to the formation of porous structure on CoP nanoflakes and regulates the electronic structure of Co through the linked O in [W–O] group as well, resultantly boosting the hydrogen production and HzOR. Moreover, a proof-of-concept direct hydrazine fuel cell-powered H2 production system has been assembled, realizing H2 evolution at a rate of 3.53 mmol cm−2 h−1 at room temperature without external electricity supply.

]]> https://link.springer.com/article/10.1007/s40820-023-01185-4 https://link.springer.com/article/10.1007/s40820-023-01185-4 Precise Detection, Control and Synthesis of Chiral Compounds at Single-Molecule Resolution

Chen Yang; Weilin Hu; Xuefeng Guo
https://doi.org/10.1007/s40820-023-01184-5
Volume 15, issue 1, December 2023

Chirality, as the symmetric breaking of molecules, plays an essential role in physical, chemical and especially biological processes, which highlights the accurate distinction among heterochiralities as well as the precise preparation for homochirality. To this end, the well-designed structure-specific recognizer and catalysis reactor are necessitated, respectively. However, each kind of target molecules requires a custom-made chiral partner and the dynamic disorder of spatial-orientation distribution of molecules at the ensemble level leads to an inefficient protocol. In this perspective article, we developed a universal strategy capable of realizing the chirality detection and control by the external symmetry breaking based on the alignment of the molecular frame to external stimuli. Specifically, in combination with the discussion about the relationship among the chirality (molecule), spin (electron) and polarization (photon), i.e., the three natural symmetry breaking, single-molecule junctions were proposed to achieve a single-molecule/event-resolved detection and synthesis. The fixation of the molecular orientation and the CMOS-compatibility provide an efficient interface to achieve the external input of symmetry breaking. This perspective is believed to offer more efficient applications in accurate chirality detection and precise asymmetric synthesis via the close collaboration of chemists, physicists, materials scientists, and engineers.

]]> https://link.springer.com/article/10.1007/s40820-023-01184-5 https://link.springer.com/article/10.1007/s40820-023-01184-5 Dual-Doped Nickel Sulfide for Electro-Upgrading Polyethylene Terephthalate into Valuable Chemicals and Hydrogen Fuel

Zhijie Chen; Renji Zheng; Bing-Jie Ni
https://doi.org/10.1007/s40820-023-01181-8
Volume 15, issue 1, December 2023

Electro-upcycling of plastic waste into value-added chemicals/fuels is an attractive and sustainable way for plastic waste management. Recently, electrocatalytically converting polyethylene terephthalate (PET) into formate and hydrogen has aroused great interest, while developing low-cost catalysts with high efficiency and selectivity for the central ethylene glycol (PET monomer) oxidation reaction (EGOR) remains a challenge. Herein, a high-performance nickel sulfide catalyst for plastic waste electro-upcycling is designed by a cobalt and chloride co-doping strategy. Benefiting from the interconnected ultrathin nanosheet architecture, dual dopants induced up-shifting d band centre and facilitated in situ structural reconstruction, the Co and Cl co-doped Ni3S2 (Co, Cl-NiS) outperforms the single-doped and undoped analogues for EGOR. The self-evolved sulfide@oxyhydroxide heterostructure catalyzes EG-to-formate conversion with high Faradic efficiency (> 92%) and selectivity (> 91%) at high current densities (> 400 mA cm−2). Besides producing formate, the bifunctional Co, Cl-NiS-assisted PET hydrolysate electrolyzer can achieve a high hydrogen production rate of 50.26 mmol h−1 in 2 M KOH, at 1.7 V. This study not only demonstrates a dual-doping strategy to engineer cost-effective bifunctional catalysts for electrochemical conversion processes, but also provides a green and sustainable way for plastic waste upcycling and simultaneous energy-saving hydrogen production.

]]> https://link.springer.com/article/10.1007/s40820-023-01181-8 https://link.springer.com/article/10.1007/s40820-023-01181-8 Zinc–Bromine Rechargeable Batteries: From Device Configuration, Electrochemistry, Material to Performance Evaluation

Norah S. Alghamdi; Masud Rana; Bin Luo
https://doi.org/10.1007/s40820-023-01174-7
Volume 15, issue 1, December 2023

Zinc–bromine rechargeable batteries (ZBRBs) are one of the most powerful candidates for next-generation energy storage due to their potentially lower material cost, deep discharge capability, non-flammable electrolytes, relatively long lifetime and good reversibility. However, many opportunities remain to improve the efficiency and stability of these batteries for long-life operation. Here, we discuss the device configurations, working mechanisms and performance evaluation of ZBRBs. Both non-flow (static) and flow-type cells are highlighted in detail in this review. The fundamental electrochemical aspects, including the key challenges and promising solutions, are discussed, with particular attention paid to zinc and bromine half-cells, as their performance plays a critical role in determining the electrochemical performance of the battery system. The following sections examine the key performance metrics of ZBRBs and assessment methods using various ex situ and in situ/operando techniques. The review concludes with insights into future developments and prospects for high-performance ZBRBs.

]]> https://link.springer.com/article/10.1007/s40820-023-01174-7 https://link.springer.com/article/10.1007/s40820-023-01174-7 Recent Advances in Structural Optimization and Surface Modification on Current Collectors for High-Performance Zinc Anode: Principles, Strategies, and Challenges

Yuxin Gong; Bo Wang; Shixue Dou
https://doi.org/10.1007/s40820-023-01177-4
Volume 15, issue 1, December 2023

The mechanisms of the surface modification and structure design of zinc anode current collectors were summarized. The recent advances of high-performance zinc anode current collectors were reviewed and categorized according to their working mechanisms. The possible prospects and directions of zinc anode research were discussed.

]]> https://link.springer.com/article/10.1007/s40820-023-01177-4 https://link.springer.com/article/10.1007/s40820-023-01177-4 Achieving Tunable Cold/Warm White-Light Emission in a Single Perovskite Material with Near-Unity Photoluminescence Quantum Yield

Bo Zhou; Aixuan Du; Yumeng Shi
https://doi.org/10.1007/s40820-023-01168-5
Volume 15, issue 1, December 2023

Single materials that exhibit efficient and stable white-light emission are highly desirable for lighting applications. This paper reports a novel zero-dimensional perovskite, Rb4CdCl6:Sn2+, Mn2+, which demonstrates exceptional white-light properties including adjustable correlated color temperature, high color rendering index of up to 85, and near-unity photoluminescence quantum yield of 99%. Using a co-doping strategy involving Sn2+ and Mn2+, cyan-orange dual-band emission with complementary spectral ranges is activated by the self-trapped excitons and d-d transitions of the Sn2+ and Mn2+ centers in the Rb4CdCl6 host, respectively. Intriguingly, although Mn2+ ions doped in Rb4CdCl6 are difficult to excite, efficient Mn2+ emission can be realized through an ultra-high-efficient energy transfer between Sn2+ and Mn2+ via the formation of adjacent exchange-coupled Sn–Mn pairs. Benefiting from this efficient Dexter energy transfer process, the dual emission shares the same optimal excitation wavelengths of the Sn2+ centers and suppresses the non-radiative vibration relaxation significantly. Moreover, the relative intensities of the dual-emission components can be modulated flexibly by adjusting the fraction of the Sn2+ ions to the Sn–Mn pairs. This co-doping approach involving short-range energy transfer represents a promising avenue for achieving high-quality white light within a single material.

]]> https://link.springer.com/article/10.1007/s40820-023-01168-5 https://link.springer.com/article/10.1007/s40820-023-01168-5 Progress and Challenges Toward Effective Flexible Perovskite Solar Cells

Xiongjie Li; Haixuan Yu; Mingkui Wang
https://doi.org/10.1007/s40820-023-01165-8
Volume 15, issue 1, December 2023

The demand for building-integrated photovoltaics and portable energy systems based on flexible photovoltaic technology such as perovskite embedded with exceptional flexibility and a superior power-to-mass ratio is enormous. The photoactive layer, i.e., the perovskite thin film, as a critical component of flexible perovskite solar cells (F-PSCs), still faces long-term stability issues when deformation occurs due to encountering temperature changes that also affect intrinsic rigidity. This literature investigation summarizes the main factors responsible for the rapid destruction of F-PSCs. We focus on long-term mechanical stability of F-PSCs together with the recent research protocols for improving this performance. Furthermore, we specify the progress in F-PSCs concerning precise design strategies of the functional layer to enhance the flexural endurance of perovskite films, such as internal stress engineering, grain boundary modification, self-healing strategy, and crystallization regulation. The existing challenges of oxygen-moisture stability and advanced encapsulation technologies of F-PSCs are also discussed. As concluding remarks, we propose our viewpoints on the large-scale commercial application of F-PSCs.

]]> https://link.springer.com/article/10.1007/s40820-023-01165-8 https://link.springer.com/article/10.1007/s40820-023-01165-8 Synergistic “Anchor-Capture” Enabled by Amino and Carboxyl for Constructing Robust Interface of Zn Anode

Zhen Luo; Yufan Xia; Yinzhu Jiang
https://doi.org/10.1007/s40820-023-01171-w
Volume 15, issue 1, December 2023

The synergistic “anchor-capture” mechanism of polar groups on Zn stripping/plating process is firstly proposed. The amino group firmly anchors on Zn surface and the carboxyl group strongly captures Zn2+, constructing a robust anode–electrolyte interface and inducing uniform Zn deposition. The ultra-stable cycle lifespan of Zn–Zn symmetric cell (over 2800 h) and high utilization rate of Zn anode (the depth of discharge up to 68% for 200 h) are achieved under the proposal of synergistic “anchor-capture.”

]]> https://link.springer.com/article/10.1007/s40820-023-01171-w https://link.springer.com/article/10.1007/s40820-023-01171-w Integration of Multiple Heterointerfaces in a Hierarchical 0D@2D@1D Structure for Lightweight, Flexible, and Hydrophobic Multifunctional Electromagnetic Protective Fabrics

Shuo Zhang; Xuehua Liu; Guanglei Wu
https://doi.org/10.1007/s40820-023-01179-2
Volume 15, issue 1, December 2023

The development of wearable multifunctional electromagnetic protective fabrics with multifunctional, low cost, and high efficiency remains a challenge. Here, inspired by the unique flower branch shape of “Thunberg’s meadowsweet” in nature, a nanofibrous composite membrane with hierarchical structure was constructed. Integrating sophisticated 0D@2D@1D hierarchical structures with multiple heterointerfaces can fully unleash the multifunctional application potential of composite membrane. The targeted induction method was used to precisely regulate the formation site and morphology of the metal–organic framework precursor, and intelligently integrate multiple heterostructures to enhance dielectric polarization, which improves the impedance matching and loss mechanisms of the electromagnetic wave absorbing materials. Due to the synergistic enhancement of electrospinning-derived carbon nanofiber “stems”, MOF-derived carbon nanosheet “petals” and transition metal selenide nano-particle “stamens”, the CoxSey/NiSe@CNSs@CNFs (CNCC) composite membrane obtains a minimum reflection loss value (RLmin) of -68.40 dB at 2.6 mm and a maximum effective absorption bandwidth (EAB) of 8.88 GHz at a thin thickness of 2.0 mm with a filling amount of only 5 wt%. In addition, the multi-component and hierarchical heterostructure endow the fibrous membrane with excellent flexibility, water resistance, thermal management, and other multifunctional properties. This work provides unique perspectives for the precise design and rational application of multifunctional fabrics.

]]> https://link.springer.com/article/10.1007/s40820-023-01179-2 https://link.springer.com/article/10.1007/s40820-023-01179-2 Nanoengineering Metal–Organic Frameworks and Derivatives for Electrosynthesis of Ammonia

Daming Feng; Lixue Zhou; Fengxia Wei
https://doi.org/10.1007/s40820-023-01169-4
Volume 15, issue 1, December 2023

Recent advances in the metal–organic framework (MOF)-related catalysts for electrochemical ammonia synthesis protocols under ambient reaction conditions are summarized and discussed. The design and fabrication of efficient electrocatalysts from MOF for the reduction of N2 and NO3− are systematically analyzed. Based on the current advances, the ongoing challenges and promising perspectives are highlighted.

]]> https://link.springer.com/article/10.1007/s40820-023-01169-4 https://link.springer.com/article/10.1007/s40820-023-01169-4 High-Quality Epitaxial N Doped Graphene on SiC with Tunable Interfacial Interactions via Electron/Ion Bridges for Stable Lithium-Ion Storage

Changlong Sun; Xin Xu; Jiahai Wang
https://doi.org/10.1007/s40820-023-01175-6
Volume 15, issue 1, December 2023

The intimate NG@SiC heterostructure has been constructed via a direct thermal decomposition method. The NG@SiC heterostructure anode delivers enhanced capacity and cycling stability both in the half-cell and in the full cell. DFT analysis reveals that this NG@SiC anode possesses lower lithium-ion adsorption energy and higher charge and discharge rates.

]]> https://link.springer.com/article/10.1007/s40820-023-01175-6 https://link.springer.com/article/10.1007/s40820-023-01175-6 Cerium Methacrylate Assisted Preparation of Highly Thermally Conductive and Anticorrosive Multifunctional Coatings for Heat Conduction Metals Protection

Fei Xu; Peng Ye; Huaiyuan Wang
https://doi.org/10.1007/s40820-023-01163-w
Volume 15, issue 1, December 2023

Preparing polymeric coatings with well corrosion resistance and high thermal conductivity (TC) to prolong operational life and ensure service reliability of heat conductive metallic materials has long been a substantive and urgent need while a difficult task. Here we report a multifunctional epoxy composite coating (F-CB/CEP) by synthesizing cerium methacrylate and ingeniously using it as a novel curing agent with corrosion inhibit for epoxy resin and modifier for boron nitride through "cation-π" interaction. The prepared F-CB/CEP coating presents a high TC of 4.29 W m−1 K−1, which is much higher than other reported anti-corrosion polymer coatings and thereby endowing metal materials coated by this coating with outstanding thermal management performance compared with those coated by pure epoxy coating. Meanwhile, the low-frequency impedance remains at 5.1 × 1011 Ω cm2 even after 181 days of immersion in 3.5 wt% NaCl solution. Besides, the coating also exhibits well hydrophobicity, self-cleaning properties, temperature resistance and adhesion. This work provides valuable insights for the preparation of high-performance composite coatings with potential to be used as advanced multifunctional thermal management materials, especially for heat conduction metals protection.

]]> https://link.springer.com/article/10.1007/s40820-023-01163-w https://link.springer.com/article/10.1007/s40820-023-01163-w Trimming the Degrees of Freedom via a K+ Flux Rectifier for Safe and Long-Life Potassium-Ion Batteries

Xianhui Yi; Apparao M. Rao; Bingan Lu
https://doi.org/10.1007/s40820-023-01178-3
Volume 15, issue 1, December 2023

High Coulombic efficiency of over 99% for dendrite-free K||Cu cell after 820 cycles. Year-scale-cycling performance of organic PTCDI cathode over 2,100 cycles. Flexible device demonstration such as fibre cell still could operate when cut into three fibre cells.

]]> https://link.springer.com/article/10.1007/s40820-023-01178-3 https://link.springer.com/article/10.1007/s40820-023-01178-3 Conformal Human–Machine Integration Using Highly Bending-Insensitive, Unpixelated, and Waterproof Epidermal Electronics Toward Metaverse

Chao Wei; Wansheng Lin; Zhong Chen
https://doi.org/10.1007/s40820-023-01176-5
Volume 15, issue 1, December 2023

The addressable electrical contact structure enables the multifunctional epidermal interface with an all-in-one function of sense, recognition, and transmission, which realizes high flexibility and high-precision touch detection. The multifunctional epidermal interface achieves superior waterproofness and is constructed enough thin to be bent freely, which is not as rigid, bulky, and thick as common interactive electronic device. The bending-insensitive characteristic facilitates accurate and stable human–machine interactions, which provides a key foundation for intelligent prostheses and super-soft robots.

]]> https://link.springer.com/article/10.1007/s40820-023-01176-5 https://link.springer.com/article/10.1007/s40820-023-01176-5 Maximizing Terahertz Energy Absorption with MXene Absorber

Xinliang Li; Hao Luo
https://doi.org/10.1007/s40820-023-01167-6
Volume 15, issue 1, December 2023

Achieving high absorption in broad terahertz bands has long been challenging for terahertz electromagnetic wave absorbers. Recently in Nature Photonics, Xiao et al. reported the high absorption approaching the theoretical upper limit across the whole terahertz band of MXene-based terahertz absorbers and, on this basis, constructed an applicable, updated alternating current impedance matching model.

]]> https://link.springer.com/article/10.1007/s40820-023-01167-6 https://link.springer.com/article/10.1007/s40820-023-01167-6 Bioorthogonal Engineered Virus-Like Nanoparticles for Efficient Gene Therapy

Chun-Jie Bao; Jia-Lun Duan; Wan-Liang Lu
https://doi.org/10.1007/s40820-023-01153-y
Volume 15, issue 1, December 2023

AbstractSection Highlights A virus-like nanoparticle (reBiosome) was developed via site-specific codon mutation for displaying unnatural amino acid (Azi) on virus envelope protein at a rational site, followed by conjugating weak acid-responsive polyethylene glycol polymer on Azi via bioorthogonal chemistry. The reBiosome exhibited reduced virus-like immunogenicity, prolonged blood circulation and enhanced delivery to weakly acidic disease foci. The reBiosome enabled efficient delivery of gene editing and gene silencing system, demonstrating remarkable therapeutic efficacy in breast cancer and arthritis, respectively.

]]> https://link.springer.com/article/10.1007/s40820-023-01153-y https://link.springer.com/article/10.1007/s40820-023-01153-y Swift Assembly of Adaptive Thermocell Arrays for Device-Level Healable and Energy-Autonomous Motion Sensors

Xin Lu; Daibin Xie; Zhuoxin Liu
https://doi.org/10.1007/s40820-023-01170-x
Volume 15, issue 1, December 2023

The MXene-boosted rapid gelling expedites the assembly of flexible thermocell arrays, overcoming the typical constraint of complicated device fabrication processes. The hydrogel electrolyte can sustain stable thermoelectrochemical performance under various challenging conditions, including large, repeated, and sustained deformations, and multiple cut-healing cycles. The as-assembled thermocell array exhibits device-level self-healing capability and high adaptability to human body, efficiently harvesting low-grade heat for wearable applications.

]]> https://link.springer.com/article/10.1007/s40820-023-01170-x https://link.springer.com/article/10.1007/s40820-023-01170-x Competitive Redox Chemistries in Vanadium Niobium Oxide for Ultrafast and Durable Lithium Storage

Xiaobo Ding; Jianhao Lin; Xunhui Xiong
https://doi.org/10.1007/s40820-023-01172-9
Volume 15, issue 1, December 2023

The over-reduction from Nb5+ to Nb3+ in the lithiation process have been demonstrated to be the critical reason for the capacity decay of Nb2O5 for the first time. A novel competitive redox strategy has been proposed to suppress the over-reduction of Nb5+ to Nb3+, which can be achieved by the incorporation of vanadium to form a new rutile VNbO4 anode. The performance of VNbO4 anode designed in this study stands among the best in cycle stability.

]]> https://link.springer.com/article/10.1007/s40820-023-01172-9 https://link.springer.com/article/10.1007/s40820-023-01172-9 Multifunctional MXene/C Aerogels for Enhanced Microwave Absorption and Thermal Insulation

Fushuo Wu; Peiying Hu; ZhengMing Sun
https://doi.org/10.1007/s40820-023-01158-7
Volume 15, issue 1, December 2023

Curving 2D MXene into 1D nanofibers can effectively stop the restacking of MXene flakes, and then the nanofibers are used to construct a lightweight and multifunctional MXene/C aerogel. The MXene/C aerogels achieved an RLmin of − 53.02 dB and EAB of 5.3 GHz. The radar cross-sectional reduction value of MXene/C aerogels can reach 12.02 dB m2. Integrating multiple functions such as thermal insulation, sensing, and microwave absorption into one material—MXene/C aerogel.

]]> https://link.springer.com/article/10.1007/s40820-023-01158-7 https://link.springer.com/article/10.1007/s40820-023-01158-7 Highly Selective Electrocatalytic CuEDTA Reduction by MoS2 Nanosheets for Efficient Pollutant Removal and Simultaneous Electric Power Output

Hehe Qin; Xinru Liu; Shun Mao
https://doi.org/10.1007/s40820-023-01166-7
Volume 15, issue 1, December 2023

Highly efficient CuEDTA removal by an electrolyzer with MoS2 nanosheet cathode. Higher removal rate and Faraday efficiency compared with other widely reported electrocatalytic technologies. CuEDTA/Zn primary battery is constructed for the first time to realize CuEDTA removal and synchronous power generation.

]]> https://link.springer.com/article/10.1007/s40820-023-01166-7 https://link.springer.com/article/10.1007/s40820-023-01166-7 Advances in Mn-Based Electrode Materials for Aqueous Sodium-Ion Batteries

Changsheng Ding; Zhang Chen; Yanfeng Gao
https://doi.org/10.1007/s40820-023-01162-x
Volume 15, issue 1, December 2023

Mn-based electrode materials, including oxides, Prussian blue analogues and polyanion compounds, are introduced systematically for aqueous sodium-ion batteries. The composition, crystal structure, morphology and electrochemical performance of Mn-based electrode materials are reviewed. The improvement methods of electrochemical performance, such as electrolyte optimization, element doping or substitution, morphology optimization and carbon modification, are discussed.

]]> https://link.springer.com/article/10.1007/s40820-023-01162-x https://link.springer.com/article/10.1007/s40820-023-01162-x Flash-Induced High-Throughput Porous Graphene via Synergistic Photo-Effects for Electromagnetic Interference Shielding

Jin Soo Lee; Jeong-Wook Kim; Keon Jae Lee
https://doi.org/10.1007/s40820-023-01157-8
Volume 15, issue 1, December 2023

AbstractSection Highlights Flash-induced porous graphene (FPG) was synthesized via a broad-spectrum flash lamp that induced synergistic photo-effects between ultraviolet and visible-near-infrared wavelengths, resulting in large-area synthesis in just a few milliseconds. A hollow pillar graphene with low sheet resistance of 18 Ω sq−1 was produced, exhibiting low density (0.0354 g cm−3) and outstanding absolute electromagnetic interference shielding effectiveness of 1.12 × 105 dB cm2 g−1. A lightweight, flexible, and high-throughput FPG is applied for electromagnetic interference shielding of a drone radar system and the human body.

]]> https://link.springer.com/article/10.1007/s40820-023-01157-8 https://link.springer.com/article/10.1007/s40820-023-01157-8 Optimized Electronic Modification of S-Doped CuO Induced by Oxidative Reconstruction for Coupling Glycerol Electrooxidation with Hydrogen Evolution

Ruo-Yao Fan; Xue-Jun Zhai; Bin Dong
https://doi.org/10.1007/s40820-023-01159-6
Volume 15, issue 1, December 2023

S-doped CuO nanorod arrays (S-CuO/CF) constructed by sulfur leaching and oxidative remodeling strategy require only 1.23 and 1.33 V versus hydrogen evolution reaction (HER) to provide glycerol oxidation currents of 100 and 500 mA cm−2. S-CuO/CF shows satisfactory performance (at 100 mA cm−2, Vcell = 1.37 V) assembled as the anode in asymmetric coupled electrolytic cell of glycerol oxidation reaction and HER. The study identifies the key factors involved in the GOR reaction pathway, which include the C–C bond breaking and lattice oxygen deintercalation steps.
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```rss https://www.springer.com/journal/41114 RSSHub i@diygod.me (DIYgod) zh-cn Tue, 10 Oct 2023 12:53:21 GMT 5 Cosmology with the Laser Interferometer Space Antenna

Pierre Auclair; David Bacon; The LISA Cosmology Working Group
https://doi.org/10.1007/s41114-023-00045-2
Volume 26, issue 1, December 2023

The Laser Interferometer Space Antenna (LISA) has two scientific objectives of cosmological focus: to probe the expansion rate of the universe, and to understand stochastic gravitational-wave backgrounds and their implications for early universe and particle physics, from the MeV to the Planck scale. However, the range of potential cosmological applications of gravitational-wave observations extends well beyond these two objectives. This publication presents a summary of the state of the art in LISA cosmology, theory and methods, and identifies new opportunities to use gravitational-wave observations by LISA to probe the universe.

]]> https://link.springer.com/article/10.1007/s41114-023-00045-2 https://link.springer.com/article/10.1007/s41114-023-00045-2 Solvable models of quantum black holes: a review on Jackiw–Teitelboim gravity

Thomas G. Mertens; Gustavo J. Turiaci
https://doi.org/10.1007/s41114-023-00046-1
Volume 26, issue 1, December 2023

We review recent developments in Jackiw–Teitelboim gravity. This is a simple solvable model of quantum gravity in two dimensions (that arises e.g. from the s-wave sector of higher dimensional gravity systems with spherical symmetry). Due to its solvability, it has proven to be a fruitful toy model to analyze important questions such as the relation between black holes and chaos, the role of wormholes in black hole physics and holography, and the way in which information that falls into a black hole can be recovered.

]]> https://link.springer.com/article/10.1007/s41114-023-00046-1 https://link.springer.com/article/10.1007/s41114-023-00046-1 Searches for continuous-wave gravitational radiation

Keith Riles
https://doi.org/10.1007/s41114-023-00044-3
Volume 26, issue 1, December 2023

Now that detection of gravitational-wave signals from the coalescence of extra-galactic compact binary star mergers has become nearly routine, it is intriguing to consider other potential gravitational-wave signatures. Here we examine the prospects for discovery of continuous gravitational waves from fast-spinning neutron stars in our own galaxy and from more exotic sources. Potential continuous-wave sources are reviewed, search methodologies and results presented and prospects for imminent discovery discussed.

]]> https://link.springer.com/article/10.1007/s41114-023-00044-3 https://link.springer.com/article/10.1007/s41114-023-00044-3 Astrophysics with the Laser Interferometer Space Antenna

Pau Amaro-Seoane; Jeff Andrews; Alejandro Vigna-Gómez
https://doi.org/10.1007/s41114-022-00041-y
Volume 26, issue 1, December 2023

The Laser Interferometer Space Antenna (LISA) will be a transformative experiment for gravitational wave astronomy, and, as such, it will offer unique opportunities to address many key astrophysical questions in a completely novel way. The synergy with ground-based and space-born instruments in the electromagnetic domain, by enabling multi-messenger observations, will add further to the discovery potential of LISA. The next decade is crucial to prepare the astrophysical community for LISA’s first observations. This review outlines the extensive landscape of astrophysical theory, numerical simulations, and astronomical observations that are instrumental for modeling and interpreting the upcoming LISA datastream. To this aim, the current knowledge in three main source classes for LISA is reviewed; ultra-compact stellar-mass binaries, massive black hole binaries, and extreme or interme-diate mass ratio inspirals. The relevant astrophysical processes and the established modeling techniques are summarized. Likewise, open issues and gaps in our understanding of these sources are highlighted, along with an indication of how LISA could help making progress in the different areas. New research avenues that LISA itself, or its joint exploitation with upcoming studies in the electromagnetic domain, will enable, are also illustrated. Improvements in modeling and analysis approaches, such as the combination of numerical simulations and modern data science techniques, are discussed. This review is intended to be a starting point for using LISA as a new discovery tool for understanding our Universe.

]]> https://link.springer.com/article/10.1007/s41114-022-00041-y https://link.springer.com/article/10.1007/s41114-022-00041-y Dynamical boson stars

Steven L. Liebling; Carlos Palenzuela
https://doi.org/10.1007/s41114-023-00043-4
Volume 26, issue 1, December 2023

The idea of stable, localized bundles of energy has strong appeal as a model for particles. In the 1950s, John Wheeler envisioned such bundles as smooth configurations of electromagnetic energy that he called geons, but none were found. Instead, particle-like solutions were found in the late 1960s with the addition of a scalar field, and these were given the name boson stars. Since then, boson stars find use in a wide variety of models as sources of dark matter, as black hole mimickers, in simple models of binary systems, and as a tool in finding black holes in higher dimensions with only a single Killing vector. We discuss important varieties of boson stars, their dynamic properties, and some of their uses, concentrating on recent efforts.

]]> https://link.springer.com/article/10.1007/s41114-023-00043-4 https://link.springer.com/article/10.1007/s41114-023-00043-4 ```